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Environ Sci Technol


Title:A Laboratory Assessment of 120 Air Pollutant Emissions from Biomass and Fossil Fuel Cookstoves
Author(s):Bilsback KR; Dahlke J; Fedak KM; Good N; Hecobian A; Herckes P; L'Orange C; Mehaffy J; Sullivan A; Tryner J; Van Zyl L; Walker ES; Zhou Y; Pierce JR; Wilson A; Peel JL; Volckens J;
Address:"Department of Mechanical Engineering , Colorado State University , 1374 Campus Delivery , Fort Collins , Colorado 80523 , United States. Department of Environmental and Radiological Health Sciences , Colorado State University , 1681 Campus Delivery , Fort Collins , Colorado 80523 , United States. Department of Atmospheric Science , Colorado State University , 1371 Campus Delivery , Fort Collins , Colorado 80523 , United States. School of Molecular Sciences , Arizona State University , 1604 Campus Delivery , Tempe , Arizona 85287 , United States. Department of Statistics , Colorado State University , 1877 Campus Delivery , Fort Collins , Colorado 80523 , United States"
Journal Title:Environ Sci Technol
Year:2019
Volume:20190607
Issue:12
Page Number:7114 - 7125
DOI: 10.1021/acs.est.8b07019
ISSN/ISBN:1520-5851 (Electronic) 0013-936X (Linking)
Abstract:"Cookstoves emit many pollutants that are harmful to human health and the environment. However, most of the existing scientific literature focuses on fine particulate matter (PM(2.5)) and carbon monoxide (CO). We present an extensive data set of speciated air pollution emissions from wood, charcoal, kerosene, and liquefied petroleum gas (LPG) cookstoves. One-hundred and twenty gas- and particle-phase constituents-including organic carbon, elemental carbon (EC), ultrafine particles (10-100 nm), inorganic ions, carbohydrates, and volatile/semivolatile organic compounds (e.g., alkanes, alkenes, alkynes, aromatics, carbonyls, and polycyclic aromatic hydrocarbons (PAHs))-were measured in the exhaust from 26 stove/fuel combinations. We find that improved biomass stoves tend to reduce PM(2.5) emissions; however, certain design features (e.g., insulation or a fan) tend to increase relative levels of other coemitted pollutants (e.g., EC ultrafine particles, carbonyls, or PAHs, depending on stove type). In contrast, the pressurized kerosene and LPG stoves reduced all pollutants relative to a traditional three-stone fire (>/=93% and >/=79%, respectively). Finally, we find that PM(2.5) and CO are not strong predictors of coemitted pollutants, which is problematic because these pollutants may not be indicators of other cookstove smoke constituents (such as formaldehyde and acetaldehyde) that may be emitted at concentrations that are harmful to human health"
Keywords:*Air Pollutants Biomass Cooking *Environmental Pollutants Fossil Fuels Humans Particulate Matter;
Notes:"MedlineBilsback, Kelsey R Dahlke, Jordyn Fedak, Kristen M Good, Nicholas Hecobian, Arsineh Herckes, Pierre L'Orange, Christian Mehaffy, John Sullivan, Amy Tryner, Jessica Van Zyl, Lizette Walker, Ethan S Zhou, Yong Pierce, Jeffrey R Wilson, Ander Peel, Jennifer L Volckens, John eng Research Support, N.I.H., Extramural 2019/05/28 Environ Sci Technol. 2019 Jun 18; 53(12):7114-7125. doi: 10.1021/acs.est.8b07019. Epub 2019 Jun 7"

 
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