| Title: | "Measurement of spatial and temporal variation in volatile hazardous air pollutants in Tacoma, Washington, using a mobile membrane introduction mass spectrometry (MIMS) system" |
| Author(s): | Davey NG; Fitzpatrick CT; Etzkorn JM; Martinsen M; Crampton RS; Onstad GD; Larson TV; Yost MG; Krogh ET; Gilroy M; Himes KH; Saganic ET; Simpson CD; Gill CG; |
| Address: | "a Department of Chemistry , University of Victoria , Victoria , British Columbia , Canada" |
| Journal Title: | J Environ Sci Health A Tox Hazard Subst Environ Eng |
| DOI: | 10.1080/10934529.2014.910014 |
| ISSN/ISBN: | 1532-4117 (Electronic) 1093-4529 (Linking) |
| Abstract: | "The objective of this study was to use membrane introduction mass spectrometry (MIMS), implemented on a mobile platform, in order to provide real-time, fine-scale, temporally and spatially resolved measurements of several hazardous air pollutants. This work is important because there is now substantial evidence that fine-scale spatial and temporal variations of air pollutant concentrations are important determinants of exposure to air pollution and adverse health outcomes. The study took place in Tacoma, WA during periods of impaired air quality in the winter and summer of 2008 and 2009. Levels of fine particles were higher in winter compared to summer, and were spatially uniform across the study area. Concentrations of vapor phase pollutants measured by membrane introduction mass spectrometry (MIMS), notably benzene and toluene, had relatively uniform spatial distributions at night, but exhibited substantial spatial variation during the day-daytime levels were up to 3-fold higher at traffic-impacted locations compared to a reference site. Although no direct side-by-side comparison was made between the MIMS system and traditional fixed site monitors, the MIMS system typically reported higher concentrations of specific VOCs, particularly benzene, ethylbenzene and naphthalene, compared to annual average concentrations obtained from SUMA canisters and gas chromatographic analysis at the fixed sites" |
| Keywords: | Air Pollutants/*analysis Air Pollution/*analysis Environmental Monitoring/instrumentation/methods Hazardous Substances/*analysis Mass Spectrometry/instrumentation/methods Volatile Organic Compounds/*analysis Washington Air toxics Mims Ms/ms diesel exhaust; |
| Notes: | "MedlineDavey, Nicholas G Fitzpatrick, Cole T E Etzkorn, Jacob M Martinsen, Morten Crampton, Robert S Onstad, Gretchen D Larson, Timothy V Yost, Michael G Krogh, Erik T Gilroy, Michael Himes, Kathy H Saganic, Erik T Simpson, Christopher D Gill, Christopher G eng Research Support, U.S. Gov't, Non-P.H.S. England 2014/06/27 J Environ Sci Health A Tox Hazard Subst Environ Eng. 2014 Sep 19; 49(11):1199-208. doi: 10.1080/10934529.2014.910014" |
