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Huan Jing Ke Xue


Title:[Pollution Characteristics and Source Apportionment of Atmospheric Volatile Organic Compounds in Winter in Kaifeng City]
Author(s):Shi YQ; Zheng KY; Ding WT; Liu JP; Chen HG; Gao G; Wang LL; Wang N; Ma SL; Zheng Y; Xie SD;
Address:"College of Environmental Sciences and Engineering, Peking University, Beijing 100871, China. 3Clear Technology Co., Ltd., Beijing 100029, China. Kaifeng Ecological Environment Monitoring Command and Dispatch Center, Kaifeng 475000, China. Kaifeng Municipal Bureau of Ecology and Environment, Kaifeng 475000, China. Henan Province Ecology Environmental Monitoring Center, Zhengzhou 450000, China"
Journal Title:Huan Jing Ke Xue
Year:2023
Volume:44
Issue:4
Page Number:1933 - 1942
DOI: 10.13227/j.hjkx.202204083
ISSN/ISBN:0250-3301 (Print) 0250-3301 (Linking)
Abstract:"In order to explore the pollution characteristics and sources of atmospheric volatile organic compounds (VOCs) in winter in Kaifeng City, based on the atmospheric VOCs component data obtained from the online monitoring station of the Kaifeng Ecological and Environmental Bureau (Urban Area) from December 2021 to January 2022, the pollution characteristics of VOCs and secondary organic aerosol formation potential (SOAP) were discussed, and the sources of VOCs were analyzed by using the PMF model. The results showed that the average mass concentration of VOCs in winter in Kaifeng City was (104.71+/-48.56) mug.m(-3), and alkanes (37.7%) had the highest proportion of mass concentrations, followed by that of halohydrocarbons (23.5%), aromatics (16.8%), OVOCs (12.6%), alkenes (6.9%), and alkynes (2.6%). The averaged total SOAP contributed by VOCs was 3.18 mug.m(-3), of which aromatics contributed as much as 83.8%, followed by alkanes (11.5%). The largest anthropogenic source of VOCs in winter in Kaifeng City was solvent utilization (17.9%), followed by fuel combustion (15.9%), industrial halohydrocarbon emission (15.8%), motor vehicle emission (14.7%), organic chemical industry (14.5%), and LPG emission (13.3%); solvent utilization contributed 32.2% of the total SOAP, followed by motor vehicle emission (22.8%) and industrial halohydrocarbon emission (18.9%). It was found that reducing VOCs emissions from solvent utilization, motor vehicle emission, and industrial halohydrocarbon emission was important to control the formation of secondary organic aerosols in winter in Kaifeng City"
Keywords:Kaifeng City secondary organic aerosol formation potential (SOAP) source apportionment volatile organic compounds (VOCs) winter;
Notes:"PubMed-not-MEDLINEShi, Yu-Qi Zheng, Kai-Yun Ding, Wei-Ting Liu, Jin-Ping Chen, Hong-Guang Gao, Guang Wang, Ling-Ling Wang, Nan Ma, Shuang-Liang Zheng, Yao Xie, Shao-Dong chi English Abstract China 2023/04/12 Huan Jing Ke Xue. 2023 Apr 8; 44(4):1933-1942. doi: 10.13227/j.hjkx.202204083"

 
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