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J Environ Manage


Title:Emission behavior and impact assessment of gaseous volatile compounds in two typical rural domestic waste landfills
Author(s):Li P; Ma J; Li L; Han Y; Zheng T; Wang Y; Chai F; Liu J;
Address:"State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: pyli_st@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: jwma_st@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; National Engineering Laboratory for VOCs Pollution Control Material & Technology, University of Chinese Academy of Sciences, Beijing, 101408, PR China. Electronic address: leel@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: yphan@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: tlzheng@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: yingwang2018_st@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: fgchai_st@rcees.ac.cn. State Key Laboratory of Environmental Aquatic Chemistry, Research Center for Eco-Environmental Sciences, Chinese Academy of Sciences, Beijing, 100085, PR China; University of Chinese Academy of Sciences, Beijing, 100049, PR China. Electronic address: jxliu@rcees.ac.cn"
Journal Title:J Environ Manage
Year:2023
Volume:20221103
Issue:Pt B
Page Number:116659 -
DOI: 10.1016/j.jenvman.2022.116659
ISSN/ISBN:1095-8630 (Electronic) 0301-4797 (Linking)
Abstract:"Landfill sites are sources of gaseous volatile compounds. The dumping area (LDA) and leachate storage pool (LSP) of two typical rural domestic waste landfill sites in north China (NLF) and southwest China (SLF) were investigated. We found that 45, 46, 61 and 68 volatile organic compounds (VOC) were present in the air of NLF-LDA, NLF-LSP, SLF-LDA, and SLF-LSP, respectively. And there were 27, 29, 35 and 37 kinds of odorous compounds being detected. Oxygenated compounds (>48.88%), chlorinated compounds (>6.85%), and aromatics (>5.46%), such as organic acid, 1-chlorobutane, and benzene, were the most abundant compounds in both landfills. The SLF-LDA had the highest olfactory effect, with a corresponding total odor activity value of 29,635.39. The ozone-formation potential analysis showed that VOCs emitted from SLF landfills had significantly higher potential for ozone formation than those from NLF landfills, with ozone generation potentials of 166.02, 225.86, 2511.82, and 1615.99 mg/m(3) for the NLF-LDA, NLF-LSP, SLF-LDA, and SLF-LSP, respectively. Higher chronic toxicity and cancer risk of VOCs were found in the SLF according to method of Risk Assessment Information System. Based on the sensitivity analysis by the Monte Carlo method, concentrations of benzene, propylene oxide, propylene, trichloroethylene, and N-nitrosodiethylamine, along with exposure duration, daily exposure time, and annual exposure frequency, significantly impacted the risk levels. We provide a scientific basis, which reflects the need for controlling and reducing gaseous pollutants from landfills, particularly rural residential landfills, which may improve rural sanitation"
Keywords:*Air Pollutants/analysis Environmental Monitoring/methods Benzene Waste Disposal Facilities *Ozone/analysis *Volatile Organic Compounds/analysis China Identification Odors Priority control of pollutants Rural domestic waste landfill Volatile organic compo;
Notes:"MedlineLi, Pengyu Ma, Jiawei Li, Lin Han, Yunping Zheng, Tianlong Wang, Ying Chai, Fengguang Liu, Junxin eng England 2022/11/07 J Environ Manage. 2023 Jan 1; 325(Pt B):116659. doi: 10.1016/j.jenvman.2022.116659. Epub 2022 Nov 3"

 
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