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Chemosphere


Title:Revealing the driving effect of emissions and meteorology on PM(2.5) and O(3) trends through a new algorithmic model
Author(s):Wang D; Zhao W; Ying N; Nie L; Shao X; Zhang W; Dang H; Zhang X;
Address:"State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China. Beijing Key Laboratory of Urban Atmospheric Volatile Organic Compounds Pollution Control and Application, Beijing Municipal Research Institute of Environment Protection, Beijing, 100037, China. State Key Laboratory of Environmental Criteria and Risk Assessment, Chinese Research Academy of Environmental Sciences, Beijing, 100012, China. Electronic address: zhangxm@craes.org.cn"
Journal Title:Chemosphere
Year:2022
Volume:20220208
Issue:
Page Number:133756 -
DOI: 10.1016/j.chemosphere.2022.133756
ISSN/ISBN:1879-1298 (Electronic) 0045-6535 (Linking)
Abstract:"Quantifying the driving effect of each factor on atmospheric secondary pollutants is crucial for pollution prevention. We aim to establish a simple and accessible method to identify ozone (O(3)) and particulate matter (PM(2.5)) concentration trends induced by emissions and meteorology. The method comprises five main steps, which involve matrix construction and mutual calculations, and the whole process is demonstrated and verified by employing long-term monitoring data. With regard to the case study, O(3) and PM(2.5) concentration variance between the target and base year are respectively -4.74 and 0.20 mug/m(3) under same meteorological conditions, among which the contribution of the emissions driver and meteorological driver are respectively -5.81 and 1.07 mug/m(3) for O(3) and respectively 0.55 and -0.35 mug/m(3) for PM(2.5). Additionally, 84.45% of O(3) variance is attributable to the emissions driver in terms of relative importance, which is 52.88% for PM(2.5). The meteorological driver is further separated into atmospheric secondary reaction and regional transport. The results reveal that ongoing prevention policy for O(3) is effective; however, it needs to be further optimized for PM(2.5)"
Keywords:*Air Pollutants/analysis *Air Pollution/analysis China Environmental Monitoring Meteorology *Ozone/analysis Particulate Matter/analysis Atmospheric secondary pollutants Emission driver Meteorology driver Pollution trend;
Notes:"MedlineWang, Di Zhao, Wenjuan Ying, Na Nie, Lei Shao, Xia Zhang, Weiqi Dang, Hongyan Zhang, Xinmin eng England 2022/02/13 Chemosphere. 2022 May; 295:133756. doi: 10.1016/j.chemosphere.2022.133756. Epub 2022 Feb 8"

 
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