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Huan Jing Ke Xue


Title:[Estimating the Secondary Organic Aerosol Concentration and Source Apportionment During the Summer and Winter in the Nanjing Industrial District]
Author(s):Liu JD; An JL; Zhang YX; Shi YZ; Lin X;
Address:"Key Laboratory of Meterological Disaster, Ministry of Education, Joint International Research Laboratory of Climate and Environment Change, Collaborative Innovation Center on Forecast and Evaluation of Meterological Disasters, Key Laboratory for Aerosol-Cloud-Precipitation of China Meteorological Administration, Nanjing University of Information Science and Technology, Nanjing 210044, China. Hangzhou Environmental Monitoring Center, Hangzhou 310007, China"
Journal Title:Huan Jing Ke Xue
Year:2017
Volume:38
Issue:5
Page Number:1733 - 1742
DOI: 10.13227/j.hjkx.201610167
ISSN/ISBN:0250-3301 (Print) 0250-3301 (Linking)
Abstract:"Volatile organic compounds (VOCs) were determined by GC5000, an automatic on-line Gas Chromatography-Flame Ionization Detector. Elemental carbon (EC) and organic carbon (OC) were determined by the thermal/optical method using DRI-2001A during the periods of June 15(th)-July 15(th) 2015 and December 16(th) 2015-January 15(th) 2016. The concentration of secondary organic aerosol(SOA) was estimated by fractional aerosol coefficients (FAC) and EC tracer method. The source apportionment relied on the positive matrix factorization model (PMF). There were several conclusions:First, aromatic hydrocarbon was the main substance causing the SOA pollution in the Nanjing Industrial district, the contributions of aromatic hydrocarbon to SOA during summer and winter were 80.39% and 94.63%, respectively. The main contributers were benzene, toluene, ethylbenzene, m,p-xylene and o-xylene (BTEX). In the summer, SOA concentration ranged from 5.84-20.88 mug.m(-3) with an average of 12.15 mug.m(-3) and in the winter ranged from 2.17-17.73 mug.m(-3) in which the average concentration was 6.91 mug.m(-3). Secondly, SOA concentration decreased when wind and precipitation increased. By using the PMF model, a total of 7sources of SOA were determined in summer and 6 were determined in winter. There were 3 main sources in summer, including painting, petroleum processing and petrochemical industry, and the contributions to SOA were 0.65 mug.m(-3), 0.21 mug.m(-3), 0.18 mug.m(-3), respectively. In winter, the most important SOA pollution was from painting, in which the contribution was 0.94 mug.m(-3)"
Keywords:EC tracer method concentration of secondary organic aerosol fractional aerosol coefficients(FAC) positive matrix factorization model and source apportionment volatile organic compounds(VOCs);
Notes:"PubMed-not-MEDLINELiu, Jing-da An, Jun-Lin Zhang, Yu-Xin Shi, Yuan-Zhe Lin, Xu chi English Abstract China 2017/05/08 Huan Jing Ke Xue. 2017 May 8; 38(5):1733-1742. doi: 10.13227/j.hjkx.201610167"

 
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