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ACS Nano


Title:Nanoalloy Printed and Pulse-Laser Sintered Flexible Sensor Devices with Enhanced Stability and Materials Compatibility
Author(s):Zhao W; Rovere T; Weerawarne D; Osterhoudt G; Kang N; Joseph P; Luo J; Shim B; Poliks M; Zhong CJ;
Address:"daggerDepartment of Chemistry, double daggerDepartment of Physics, and section signDepartment of System Science and Industrial Engineering, State University of New York at Binghamton, Binghamton, New York 13902, United States"
Journal Title:ACS Nano
Year:2015
Volume:20150602
Issue:6
Page Number:6168 - 6177
DOI: 10.1021/acsnano.5b02704
ISSN/ISBN:1936-086X (Electronic) 1936-0851 (Linking)
Abstract:"While conformal and wearable devices have become one of the most desired formats for printable electronics, it is challenging to establish a scalable process that produces stable conductive patterns but also uses substrates compatible with widely available wearable materials. Here, we describe findings of an investigation of a nanoalloy ink printed and pulsed-laser sintered conductive patterns as flexible functional devices with enhanced stability and materials compatibility. While nanoparticle inks are desired for printable electronics, almost all existing nanoparticle inks are based on single-metal component, which, as an electronic element, is limited by its inherent stabilities of the metal such as propensity of metal oxidation and mobility of metal ions, especially in sintering processes. The work here has demonstrated the first example in exploiting plasmonic coupling of nanoalloys and pulsed-laser energy with controllable thermal penetration. The experimental and theoretical results have revealed clear correlation between the pulsed laser parameters and the nanoalloy structural characteristics. The superior performance of the resulting flexible sensor device, upon imparting nanostructured sensing materials, for detecting volatile organic compounds has significant implications to developing stable and wearable sensors for monitoring environmental pollutants and breath biomarkers. This simple 'nanoalloy printing-laser sintering-nanostructure printing' process is entirely general to many different sensor devices and nanostructured sensing materials, enabling the ability to easily construct sophisticated sensor array"
Keywords:Alloys/*chemistry Ink *Lasers Metal Nanoparticles/*chemistry *Printing Volatile Organic Compounds/*analysis nanoalloy nanoink nanostructured sensing thin films printed electronics printed flexible device pulsed -laser sintering wearable sensor;
Notes:"MedlineZhao, Wei Rovere, Thomas Weerawarne, Darshana Osterhoudt, Gavin Kang, Ning Joseph, Pharrah Luo, Jin Shim, Bonggu Poliks, Mark Zhong, Chuan-Jian eng Research Support, Non-U.S. Gov't Research Support, U.S. Gov't, Non-P.H.S. 2015/06/03 ACS Nano. 2015 Jun 23; 9(6):6168-77. doi: 10.1021/acsnano.5b02704. Epub 2015 Jun 2"

 
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