| Title: | Low Temperature Combustion of VOCs with Enhanced Catalytic Activity Over MnO(2) Nanotubes Loaded with Pt and Ni-Fe Spinel |
| Author(s): | Wang Y; He J; Li X; Wang M; Zhou Y; Xiao J; Chen D; Lu J; |
| Address: | "College of Chemistry, Chemical Engineering and Materials Science, Collaborative Innovation Center of Suzhou Nano Science and Technology, Soochow University, Suzhou 215123, China" |
| Journal Title: | ACS Appl Mater Interfaces |
| ISSN/ISBN: | 1944-8252 (Electronic) 1944-8244 (Linking) |
| Abstract: | "MnO(2) nanotubes loaded with Pt and Ni-Fe spinel were synthesized using simple hydrothermal and sol-gel techniques. After loading with Ni-Fe spinel, the specific surface area of the material increases 3-fold. This change helped to provide more active sites and facilitated the association between the catalyst and volatile organic compounds (VOCs). X-ray photoelectron spectroscopy determined that the adsorbed oxygen concentrations were all greatly increased after Pt loading, indicating that Pt promoted the adsorption of oxygen and so accelerated the combustion process. The performance of the catalyst after loading with 2 wt % Pt was greatly improved, such that the T(90) for benzene decomposition was decreased to 113 degrees C. In addition, the 2% Pt/2Mn@NFO exhibited excellent low-temperature catalytic activity when reacting with low concentrations of toluene and ethyl acetate. This work therefore demonstrates a viable new approach to the development of Mn-based catalysts for the low temperature catalytic remediation of VOCs" |
| Keywords: | MnO2 nanotubes Ni-Fe spinel Pt nanoparticles VOCs oxidation low-temperature catalytic; |
| Notes: | "PubMed-not-MEDLINEWang, Yaru He, Jiaqin Li, Xunxun Wang, Mengmeng Zhou, Yuanbo Xiao, Jun Chen, Dongyun Lu, Jianmei eng 2021/09/22 ACS Appl Mater Interfaces. 2021 Oct 6; 13(39):46830-46839. doi: 10.1021/acsami.1c15372. Epub 2021 Sep 21" |
